Remodeling of Fumagillol: Discovery of an Oxygen-Directed Oxidative Mannich Reaction

نویسندگان

  • Alexander J. Grenning
  • John K. Snyder
  • John A. Porco
چکیده

An efficient, two-step construction of highly complex alkaloid-like compounds from the natural product fumagillol is described. This approach, which mimics a biosynthetic cyclase/oxidase sequence, allows for rapid and efficient structure elaboration of the basic fumagillol scaffold with a variety of readily available coupling partners. Mechanistic experiments leading to the discovery of an oxygen-directed oxidative Mannich reaction are also described.

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عنوان ژورنال:

دوره 16  شماره 

صفحات  -

تاریخ انتشار 2014